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Electrical double layer supercapacitors based on graphene nanoplatelets electrodes in organic and aqueous electrolytes: Effect of binders and scalable performance

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dc.contributor.authors Cetinkaya, T; Dryfe, RAW;
dc.date.accessioned 2020-10-16T11:08:50Z
dc.date.available 2020-10-16T11:08:50Z
dc.date.issued 2018
dc.identifier.citation Cetinkaya, T; Dryfe, RAW; (2018). Electrical double layer supercapacitors based on graphene nanoplatelets electrodes in organic and aqueous electrolytes: Effect of binders and scalable performance. JOURNAL OF POWER SOURCES, 408, 104-91
dc.identifier.issn 0378-7753
dc.identifier.uri https://doi.org/10.1016/j.jpowsour.2018.10.072
dc.identifier.uri https://hdl.handle.net/20.500.12619/69752
dc.description.abstract The effect of some commercial binders, carboxymethyl cellulose, polyvinylidene fluoride, modified styrene butadiene copolymer and vinylidene fluoride-hexafluoropropene copolymer on the capacitive performance of symmetric Graphene nanoplatelets (GnP) electrodes has been investigated in both organic and aqueous electrolytes. Surface area, pore size distribution, resistance and wetting behaviour of the electrodes have been measured and the effects of these factors have been studied to rationalise their electrical double layer capacitor (EDLC) performances. The most homogeneous distribution and lowest aggregation of the GnP electrode is obtained with CMC binder. Among the electrodes, it has also shown better capacitive behaviour in both aqueous and organic electrolyte due to its higher surface area, and higher mesoporous and microporous distributions than the other electrodes. To investigate scalable performance of the GnP electrodes, CMC binder electrodes have been scaled up from coin cell to pouch cell size. The coin cell electrodes showed higher capacitance than the pouch cell up to current densities of 50 A g(-1). The pouch cell has exhibited the higher capacitance at 50 A g(-1) and better capacitance retention, which shows that the pouch cell is a better charge storage device than coin cell at high current densities.
dc.language English
dc.publisher ELSEVIER SCIENCE BV
dc.subject Materials Science
dc.title Electrical double layer supercapacitors based on graphene nanoplatelets electrodes in organic and aqueous electrolytes: Effect of binders and scalable performance
dc.type Article
dc.identifier.volume 408
dc.identifier.startpage 91
dc.identifier.endpage 104
dc.contributor.department Sakarya Üniversitesi/Mühendislik Fakültesi/Metalurji Ve Malzeme Mühendisliği Bölümü
dc.contributor.saüauthor Çetinkaya, Tuğrul
dc.relation.journal JOURNAL OF POWER SOURCES
dc.identifier.wos WOS:000451936200012
dc.identifier.doi 10.1016/j.jpowsour.2018.10.072
dc.identifier.eissn 1873-2755
dc.contributor.author Çetinkaya, Tuğrul
dc.contributor.author Robert A. W. Dryfe


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